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Abstract of [Budewig22]

[Budewig22]
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Theoretical investigation of orbital alignment of x-ray-ionized atoms in exotic electronic configurations

Laura Budewig, Sang-Kil Son, and Robin Santra

Phys. Rev. A 105, 033111 (2022)

[bib][BibTeX][pdf][pdf][link]doi:10.1103/PhysRevA.105.033111

We theoretically study orbital alignment in x-ray-ionized atoms and ions, based on improved electronic-structure calculations starting from the Hartree-Fock-Slater model. We employ first-order many-body perturbation theory to improve the Hartree-Fock-Slater calculations and show that the use of first-order-corrected energies yields significantly better transition energies than originally obtained. The improved electronic-structure calculations enable us also to compute individual state-to-state cross sections and transition rates and, thus, to investigate orbital alignment induced by linearly polarized x rays. To explore the orbital alignment of transiently formed ions after photoionization, we discuss alignment parameters and ratios of individual state-resolved photoionization cross sections for initially neutral argon and two exotic electronic configurations that may be formed during x-ray multiphoton ionization dynamics induced by x-ray free-electron lasers. We also present how the orbital alignment is affected by Auger-Meitner decay and demonstrate how it evolves during a sequence of one photoionization and one Auger-Meitner decay. Our present work establishes a step toward investigation of orbital alignment in atomic ionization driven by high-intensity x rays.

Tags: HFS, orbital alignment, Ar, Ne, XATOM, CFEL, DESY


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